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Optimization of CuIn1-XGaXS2 Nanoparticles and Their Application in the Hole-Transporting Layer of Highly Efficient and Stable Mixed-Halide Perovskite Solar Cells
, Article ACS Applied Materials and Interfaces ; Volume 11, Issue 34 , 2019 , Pages 30838-30845 ; 19448244 (ISSN) ; Marandi, M ; Khosroshahi, R ; Malekshahi Byranvand, M ; Dehghani, M ; Zad, A. I ; Tajabadi, F ; Taghavinia, N ; Sharif University of Technology
American Chemical Society
2019
Abstract
Inorganic hole-transport materials (HTMs) have been frequently applied in perovskite solar cells (PSCs) and are a promising solution to improve the poor stability of PSCs. In this study, we investigate solution-processed copper indium gallium disulfide (CIGS) nanocrystals (NCs) as a dopant-free inorganic HTM in n-i-p type PSCs. Moreover, Cs0.05(MA0.17-FA0.83)0.95Pb(I0.83Br0.17)3 mixed-halide perovskite with proper crystalline quality and long-time stability was utilized as the light-absorbing layer under ambient conditions. To optimize the cell performance and better charge extraction from the perovskite layer, the Ga concentration in the Cu(In1-XGaX)S2 composition was changed, and the X...